There is a need to find a replacement for the 252Cf sources currently used in Standards-based performance testing of neutron instrumentation. This is a result of its relatively short half-life, concerns about future availability and recent increases in cost. A potential replacement source, 244Cm is evaluated in this study where two commercially available sources have been acquired and their neutron emission spectra measured using a pair of spectrometers. Both instruments showed the 244Cm spontaneous neutron spectrum to be fully consistent with a MCNP6®-calculated spectrum using published Watt fission parameters for 244Cm. In addition, the emission rate of the weaker 244Cm source was established through a direct count rate comparison against a calibrated and similarly encapsulated 252Cf source. The 244Cm source emission rate was found to be in excellent agreement with value stated on the manufacturer's source certificate. It is concluded that 244Cm would be an ideal replacement for 252Cf based on its longer half-life (18.1 y) and its essentially identical neutron emission spectrum. In addition, 244Cm sources are commercially available at reasonable cost.

译文

:有必要寻找一种替代品,以替代当前在基于标准的中子仪器性能测试中使用的252Cf离子源。这是由于其相对较短的半衰期,对未来可用性的担忧以及最近成本的增加。在这项研究中评估了一个潜在的替代源244Cm,其中已获得了两个市售源,并使用一对光谱仪测量了它们的中子发射光谱。两种仪器均显示244Cm自发中子光谱与使用已公布的244Cm瓦特裂变参数的MCNP6®计算光谱完全一致。另外,较弱的244Cm源的发射速率是通过与校准并类似封装的252Cf源的直接计数速率比较来确定的。发现244Cm源的排放速率与制造商的源证书中规定的值高度吻合。结论是,基于244Cm的更长的半衰期(18.1 y)和基本相同的中子发射光谱,它将是252Cf的理想替代品。另外,以合理的价格可购得244Cm源。

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