Realization of electrically pumped lasing with solution processable materials will have a revolutionary impact on many disciplines including photonics, chemical sensing, and medical diagnostics. Due to readily tunable, size-controlled emission wavelengths, colloidal semiconductor quantum dots (QDs) are attractive materials for attaining this goal. Here we use specially engineered QDs to demonstrate devices that operate as both a light emitting diode (LED) and an optically pumped laser. These structures feature a distributed feedback resonator integrated into a bottom LED electrode. By carefully engineering a refractive-index profile across the device, we are able to obtain good confinement of a waveguided mode within the QD medium, which allows for demonstrating low-threshold lasing even with an ultrathin (about three QD monolayers) active layer. These devices also exhibit strong electroluminescence (EL) under electrical pumping. The conducted studies suggest that the demonstrated dual-function (lasing/EL) structures represent a promising device platform for realizing colloidal QD laser diodes.

译文

:用溶液可处理材料实现电泵浦激光技术将对包括光子学,化学传感和医学诊断在内的许多学科产生革命性的影响。由于易于调节尺寸,控制发射波长,胶体半导体量子点(QD)是实现此目标的有吸引力的材料。在这里,我们使用经过特殊设计的QD来演示既可以用作发光二极管(LED)也可以用作光泵浦激光器的设备。这些结构的特征是集成在底部LED电极中的分布式反馈谐振器。通过仔细设计整个设备的折射率分布,我们能够在QD介质中很好地限制波导模式,即使在超薄(约三个QD单层)有源层的情况下,也可以演示低阈值激光发射。这些器件在电泵浦下还具有很强的电致发光(EL)性能。进行的研究表明,已证明的双功能(激光/ EL)结构代表了实现胶体QD激光二极管的有前途的设备平台。

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