Phytochemical investigation of the roots of Salvia miltiorrhiza led to isolations of two new depsides (1-2), along with thirteen known compounds (3-15). Their structures and relative stereochemistry were elucidated by NMR spectral (1H and 13C NMR, HSQC, HMBC), CD and HR-ESIMS data analyses. The absolute configuration of 1 was determined by comparison of the experimental and calculated ECD spectra. All the depsides (1-10) were found to exhibit stronger free radical scavenging capacity (ranging from 2.62 to 22.05μM) than diterpenoids (11-15, IC50>100μM), among which Salvianolic acid A and Salvianolic acid B were the most potent compounds. Additionally, most of depsides (1, 3, 5, 7, 8, 9, 10) possessed significant protective effects against H2O2-induced H9c2 apoptosis in low concentrations. The negative mode collision-induced dissociations of compound 1 and 2 were featured by the α-cleavage and β-cleavage to lose danshensu (198Da) and caffeic acid (180Da), respectively, while α,β-dihydroxybenzenes depsides (8-hydroxy) showed characteristic neutral elimination of H2O.

译文

丹参的根的植物化学研究导致分离出两个新的糊精(1-2)以及十三种已知化合物(3-15)。通过NMR光谱(1H和13C NMR,HSQC,HMBC),CD和HR-ESIMS数据分析阐明了它们的结构和相对立体化学。通过比较实验和计算出的ECD光谱,可以确定1的绝对构型。发现所有糊精(1-10)都比二萜类化合物(11-15,IC50>100μM)表现出更强的自由基清除能力(范围为2.62至22.05μM),其中丹酚酸A和丹酚酸B最有效。化合物。另外,大多数低浓度的分散剂(1、3、5、7、8、9、10)对H2O2诱导的H9c2细胞凋亡具有显着的保护作用。化合物1和2的负模式碰撞诱导解离的特征是α裂解和β裂解分别失去了丹参素(198Da)和咖啡酸(180Da),而α,β-二羟基苯多酚(8-羟基)表现出中性消除H2O的特性。

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