Inorder to brought S-naproxen into small intestine, an optically pure (S)-naproxen starch ester was produced by lipase through enantio-selective trans-esterification of racemic naproxen methyl ester with pretreatment starch in solvent system. With carefully selection of the reaction medium (isooctane), lipase (Carica Papaya Lipase, CPL) and the reaction mode (intermittent opening), a high conversion rate (48.6%) and enantiomeric excess of product (99.6%) was obtained. The slow release macromolecular (S)-Naproxen had been synthesized to improve the efficacy of racemic naproxen and overcome its side effects. The enanitomeric ratio of CPL (E=52.5) was higher than CRL (E=22) and greatly influenced by the byproduct methyl alcohol. The intermittent opening reaction mode was the effective way to remove the inhibition of methyl alcohol and to improve the enantio-selectivity of CPL. S-naproxen starch was confirmed by HPLC and 1H NMR. This method may also apply to preparation the other optically pure 2-phenylpropionic acid derivatives. S-naproxen starch was a new optically pure derivatives possessing emulsifying and slow release properties would be widely applied to the food, pharmaceutical and biomedical industries.

译文

为了将S-萘普生带入小肠,通过脂肪酶通过外消旋萘普生甲酯与预处理淀粉在溶剂体系中的对映选择性酯化反应,制得光学纯的 (S)-萘普生淀粉酯。通过仔细选择反应介质 (异辛烷) 、脂肪酶 (番木瓜脂肪酶,CPL) 和反应模式 (间歇开放),获得高转化率 (48.6%) 和对映体过量的产物 (99.6%)。合成了缓释大分子萘普生,以提高外消旋萘普生的功效并克服其副作用。CPL的烯醇比 (E = 52.5) 高于CRL (E = 22),并且受副产物甲醇的影响很大。间歇开放反应模式是去除甲醇抑制和提高CPL对映体选择性的有效途径。通过HPLC和1H NMR证实了S-萘普生淀粉。该方法也可用于制备其他光学纯的2-苯基丙酸衍生物。S-萘普生淀粉是一种新型的光学纯衍生物,具有乳化和缓释特性,被广泛应用于食品、制药和生物医药行业。

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