Graphene aerogels with high surface areas, ultra-low densities and thermal conductivities have been prepared to exploit their wide applications from pollution adsorption to energy storage, supercapacitor, and thermal insulation. However, the low mechanical properties, poor thermal stability and electric conductivity restrict these aerogels' applications. In this paper, we prepared mechanically strong graphene aerogels with large BET surface areas, low thermal conductivities, high thermal stability and electric conductivities via hydrothermal reduction and supercritical ethanol drying. Annealing at 1500 °C resulted in slightly increased thermal conductivity and further improvement in mechanical properties, oxidation temperature and electric conductivity of the graphene aerogel. The large BET surface areas, together with strong mechanical properties, low thermal conductivities, high thermal stability and electrical conductivities made these graphene aerogels feasible candidates for use in a number of fields covering from batteries to sensors, electrodes, lightweight conductor and insulation materials.

译文

已经准备了具有高表面积,超低密度和热导率的石墨烯气凝胶,以利用其从污染吸附到储能,超级电容器和隔热的广泛应用。但是,低的机械性能,较差的热稳定性和电导率限制了这些气凝胶的应用。在本文中,我们通过水热还原和超临界乙醇干燥制备了具有大BET表面积,低热导率,高热稳定性和电导率的机械强石墨烯气凝胶。在1500 ℃ 退火导致略微增加的热导率,并进一步改善石墨烯气凝胶的机械性能、氧化温度和电导率。较大的BET表面积,以及强的机械性能,低的热导率,高热稳定性和电导率,使得这些石墨烯气凝胶可用于从电池到传感器,电极,轻质导体和绝缘材料的许多领域。

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