We studied the charge recombination characteristics of Photosystem II (PSII) redox components in whole cells of the chlorophyll (Chl) d-dominated cyanobacterium, Acaryochloris marina, by flash-induced chlorophyll fluorescence and thermoluminescence measurements. Flash-induced chlorophyll fluorescence decay was retarded in the mus and ms time ranges and accelerated in the s time range in Acaryochloris marina relative to that in the Chl a-containing cyanobacterium, Synechocystis PCC 6803. In the presence of 3-(3,4-dichlorophenyl)-1, 1-dimethylurea, which blocks the Q(B) site, the relaxation of fluorescence decay arising from S(2)Q(A)(-) recombination was somewhat faster in Acaryochloris marina than in Synechocystis PCC 6803. Thermoluminescence intensity of the so called B band, arising from the recombination of the S(2)Q(B)(-) charge separated state, was enhanced significantly (2.5 fold) on the basis of equal amounts of PSII in Acaryochloris marina as compared with Synechocystis 6803. Our data show that the energetics of charge recombination is modified in Acaryochloris marina leading to a approximately 15 meV decrease of the free energy gap between the Q(A) and Q(B) acceptors. In addition, the total free energy gap between the ground state and the excited state of the reaction center chlorophyll is at least approximately 25-30 meV smaller in Acaryochloris marina, suggesting that the primary donor species cannot consist entirely of Chl a in Acaryochloris marina, and there is a contribution from Chl d as well.

译文

:我们通过闪光诱导的叶绿素荧光和热致发光测量研究了叶绿素(Chl)d为主的蓝细菌,无核小球藻的整个细胞中光系统II(PSII)氧化还原组分的电荷重组特性。相对于含Chla的蓝藻细菌Synechocystis PCC 6803,在无性纲中,闪光诱导的叶绿素荧光衰减在mus和ms的时间范围内被延迟,并在s的时间范围内被加速。在存在3-(3,4 -二氯苯基)-1,1-二甲基脲,阻止Q(B)站点,由S(2)Q(A)(-)重组引起的荧光衰减的弛豫比拟蓝藻PCC 6803快一点。由于在S.2Q(B)(-)电荷分离状态的重组下产生的所谓的B带的热致发光强度与无毒双杀藻码头中等量的PSII相比显着提高了(2.5倍)与拟南芥6803。我们的数据显示,电荷重组的能量在滨蛇纲中被修饰,导致Q(A)和Q(B)受体之间的自由能隙减小了约15 meV。此外,在无核无盐藻中,基态和反应中心叶绿素的激发态之间的总自由能隙至少小25-30 meV,这表明主要供体不能完全由无性无藻中的Chla组成, Chl d也有贡献。

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