In the present study, the electrocatalytic oxidation of reduced β nicotinamide adenine dinucleotide (NADH) was investigated using a pencil graphite electrode modified with quercetin (PGE/QH(2)). The PGE/QH(2) was prepared through two steps: (i) the pre-treatment of PGE at 1.40 V vs. Ag|AgCl|KCl((sat.)) in pH 7.0 phosphate buffer containing 0.1 M KCl for 60s and (ii) adsorption of QH(2) on the PGE via immersion of PGE into a 1.0mM QH(2) solution (in ethanol) for 60s. Cyclic voltammetric studies show that the peak potential of NADH oxidation shifts from +500 mV at bare PGE to +300 mV at PGE/QH(2). The electrocatalytic currents obtained from amperometric measurements at +300 mV vs. Ag|AgCl|KCl((sat.)) and in phosphate buffer solution at pH 7.0 containing 0.1M KCl were linearly related to the concentration of NADH. Linear calibration plots are obtained in the concentration range from 0.5 μM to 100 μM. The limit of detection was found to be 0.15 μM.

译文

在本研究中,使用槲皮素 (PGE/QH(2)) 修饰的铅笔石墨电极研究了还原的 β 烟酰胺腺嘌呤二核苷酸 (NADH) 的电催化氧化。通过两个步骤制备PGE/QH(2): (i) 在含有0.1 M KCl的pH 7.0磷酸盐缓冲液中1.40 V对Ag | AgCl | KCl((sat。)) 预处理60s,以及 (ii) 通过将PGE浸入1.0毫米QH(2) 在PGE上吸附QH(2)) 溶液 (在乙醇中) 60s。循环伏安研究表明,NADH氧化的峰电位从裸露PGE处的 + 500 mV转变为PGE/QH(2) 处的 + 300 mV。从在 + 300 mV对Ag | AgCl | KCl((sat。)) 和在含有0.1M KCl的pH 7.0的磷酸盐缓冲溶液中的安培测量获得的电催化电流与NADH的浓度线性相关。在从0.5微米到100微米的浓度范围内获得线性校准图。发现检出限为0.15微米。

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