D-configured poly(D-lactic acid) (D-PLA) and poly(D-2-hydroxy-3-methylbutanoic acid) (D-P2H3MB) crystallized separately into their homo-crystallites when crystallized by precipitation or solvent evaporation, whereas incorporation of L-configured poly(L-2-hydroxybutanoic acid) (L-P2HB) in D-configured D-PLA and D-P2H3MB induced co-crystallization or ternary stereocomplex formation between D-configured D-PLA and D-P2H3MB and L-configured L-P2HB. However, incorporation of D-configured poly(D-2-hydroxybutanoic acid) (D-P2HB) in D-configured D-PLA and D-P2H3MB did not cause co-crystallization between D-configured D-PLA and D-P2H3MB and D-configured D-P2HB but separate crystallization of each polymer occurred. These findings strongly suggest that an optically active polymer (L-configured or D-configured polymer) like unsubstituted or substituted optically active poly(lactic acid)s can act as "a configurational or helical molecular glue" for two oppositely configured optically active polymers (two D-configured polymers or two L-configured polymers) to allow their co-crystallization. The increased degree of freedom in polymer combination is expected to assist to pave the way for designing polymeric composites having a wide variety of physical properties, biodegradation rate and behavior in the case of biodegradable polymers.

译文

D型聚 (D-乳酸) (D-PLA) 和聚 (D-2-hydroxy-3-methylbutanoic) (D-P2H3MB) 在通过沉淀或溶剂蒸发结晶时分别结晶成其同型微晶,而将L-配置的聚 (L-2-hydroxybutanoic) (L-P2HB) 掺入D-配置的D-PLA中并D-P2H3MB诱导D-配置的D-PLA与D-P2H3MB和L-配置的L-P2HB之间的共结晶或三元立体复合物形成。然而,D-配置的聚 (D-2-hydroxybutanoic) (D-P2HB) 在D-配置的D-PLA和D-P2H3MB中的掺入不会引起D-配置的D-PLA与D-P2H3MB和D-配置的D-P2HB之间的共结晶,但是发生了每种聚合物的单独结晶。这些发现强烈表明,光学活性聚合物 (L型或D型聚合物) (如未取代或取代的光学活性聚乳酸) 可以充当两种相反配置的光学活性聚合物 (两种D型聚合物或两种L型聚合物) 的 “构型或螺旋分子胶” 聚合物) 以使其共结晶。聚合物组合中增加的自由度有望有助于为设计具有多种物理性能,生物降解速率和在可生物降解聚合物的情况下的行为的聚合物复合材料铺平道路。

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