The metabolism of the reproductive and developmental toxicant bis(2-methoxyethyl)ether (diglyme) was studied in isolated rat hepatocytes and in the intact rat. Male Sprague-Dawley rats (190-220 g) were used in both studies. Hepatocytes, isolated by a two-step in situ collagenase perfusion of the liver, were cultured as monolayers and incubated with [14C]diglyme at 1, 10, 30, and 50 microM for up to 48 h. For the in vivo study, rats were given single oral doses of [14C]diglyme at 5.1 mmol/kg body wt, and urine was collected for up to 96 h. Radioactive compounds in the culture medium or in the urine were separated by high performance liquid chromatography and quantified with an in-line radioactivity monitor. Metabolites were identified by comparison of their chromatographic retention times and their mass spectra with those of authentic compounds. The principal metabolite from hepatocytes and in the urine was (2-methoxyethoxy)acetic acid (MEAA). This metabolite accounted for approximately 36% of the radioactivity in the 48-h culture medium and about 67% of the administered dose in the 48-h urine. Other prominent metabolites common to both systems included 2-(2-methoxyethoxy)ethanol, methoxyacetic acid (MAA), 2-methoxyethanol, and diglycolic acid. The diglyme metabolite profiles from urine and from hepatocytes were qualitatively similar, demonstrating that, in the rat, hepatocytes serve as a good model system for predicting the urinary metabolites of diglyme. Moreover, MEAA was shown to be the metabolite best suited for use as a short-term biological marker of exposure to diglyme.(ABSTRACT TRUNCATED AT 250 WORDS)

译文

在分离的大鼠肝细胞和完整的大鼠中研究了生殖和发育毒性双 (2-甲氧基乙基) 醚 (dlyme) 的代谢。两项研究中都使用了雄性Sprague-Dawley大鼠 (190-220g)。肝细胞,通过肝脏的两步原位胶原酶灌注分离,以单层培养,并与 [14C] 二甘醇在1、10、30和50微米下孵育长达48小时。对于体内研究,给大鼠单次口服剂量为5.1 mmol/kg体重的 [14C] 二甘醇,收集尿液长达96小时。培养基或尿液中的放射性化合物通过高效液相色谱分离,并用在线放射性监测仪定量。通过将其色谱保留时间和质谱与真实化合物进行比较来鉴定代谢物。主要代谢物来自肝细胞和尿液中的是 (2-甲氧基乙氧基) 乙酸 (MEAA)。这种代谢物约占48小时培养基中放射性的36%,约占48小时尿液中给药剂量的67%。这两个系统常见的其他突出代谢物包括2-(2-甲氧基乙氧基) 乙醇,甲氧基乙酸 (MAA),2-甲氧基乙醇和二乙醇酸。尿液和肝细胞的二甘醇胺代谢物谱在定性上相似,表明在大鼠中,肝细胞是预测二甘醇胺尿代谢物的良好模型系统。此外,MEAA被证明是最适合用作暴露于dlyme的短期生物标志物的代谢物。(摘要截短于250字)

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